Ultrafast Terahertz Gating of the Polarization and Giant Nonlinear Optical Response in BiFeO3 Thin Films.

نویسندگان

  • Frank Chen
  • John Goodfellow
  • Shi Liu
  • Ilya Grinberg
  • Matthias C Hoffmann
  • Anoop R Damodaran
  • Yi Zhu
  • Peter Zalden
  • Xiaohang Zhang
  • Ichiro Takeuchi
  • Andrew M Rappe
  • Lane W Martin
  • Haidan Wen
  • Aaron M Lindenberg
چکیده

Terahertz pulses are applied as an all-optical bias to ferroelectric thin-film BiFeO3 while monitoring the time-dependent ferroelectric polarization through its nonlinear optical response. Modulations in the intensity of the second harmonic light generated by the film correspond to on-off ratios of 220× gateable on femtosecond timescales. Polarization modulations comparable to the built-in static polarization are observed.

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عنوان ژورنال:
  • Advanced materials

دوره 27 41  شماره 

صفحات  -

تاریخ انتشار 2015